The formation of defect-pairs for highly efficient visible-light catalysts

Qingbo Sun; David Cortie; Shaoyang Zhang; Terry J. Frankcombe; Guangwei She; Jie Gao; Leigh R. Sheppard; Wanbiao Hu; Hua Chen; Shangjun Zhuo; Dehong Chen; Ray L. Withers; Garry McIntyre; Dehong Yu; Wensheng Shi; Yun Liu

doi:10.1002/adma.201605123

The formation of defect-pairs for highly efficient visible-light catalysts

Qingbo Sun, David Cortie, Shaoyang Zhang, Terry J. Frankcombe, Guangwei She, Jie Gao, Leigh R. Sheppard, Wanbiao Hu, Hua Chen, Shangjun Zhuo, Dehong Chen, Ray L. Withers, Garry McIntyre, Dehong Yu, Wensheng Shi, Yun Liu

Research output: Contribution to journal › Article › peer-review

50 Citations (Scopus)

Abstract

Highly efficient visible-light catalysts are achieved through forming defect-pairs in TiO2 nanocrystals. This study therefore proposes that fine-tuning the chemical scheme consisting of charge-compensated defect-pairs in balanced concentrations is a key missing step for realizing outstanding photocatalytic performance. This research benefits photocatalytic applications and also provides new insight into the significance of defect chemistry for functionalizing materials.

Original language	English
Article number	1605123
Number of pages	6
Journal	Advanced Materials
Volume	29
Issue number	11
DOIs	https://doi.org/10.1002/adma.201605123
Publication status	Published - 2017

Keywords

photocatalysis
solar energy
titanium dioxide
visible-light catalysts

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10.1002/adma.201605123

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title = "The formation of defect-pairs for highly efficient visible-light catalysts",

abstract = "Highly efficient visible-light catalysts are achieved through forming defect-pairs in TiO2 nanocrystals. This study therefore proposes that fine-tuning the chemical scheme consisting of charge-compensated defect-pairs in balanced concentrations is a key missing step for realizing outstanding photocatalytic performance. This research benefits photocatalytic applications and also provides new insight into the significance of defect chemistry for functionalizing materials.",

keywords = "photocatalysis, solar energy, titanium dioxide, visible-light catalysts",

author = "Qingbo Sun and David Cortie and Shaoyang Zhang and Frankcombe, {Terry J.} and Guangwei She and Jie Gao and Sheppard, {Leigh R.} and Wanbiao Hu and Hua Chen and Shangjun Zhuo and Dehong Chen and Withers, {Ray L.} and Garry McIntyre and Dehong Yu and Wensheng Shi and Yun Liu",

year = "2017",

doi = "10.1002/adma.201605123",

language = "English",

volume = "29",

journal = "Advanced Materials",

issn = "0935-9648",

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T1 - The formation of defect-pairs for highly efficient visible-light catalysts

AU - Sun, Qingbo

AU - Cortie, David

AU - Zhang, Shaoyang

AU - Frankcombe, Terry J.

AU - She, Guangwei

AU - Gao, Jie

AU - Sheppard, Leigh R.

AU - Hu, Wanbiao

AU - Chen, Hua

AU - Zhuo, Shangjun

AU - Chen, Dehong

AU - Withers, Ray L.

AU - McIntyre, Garry

AU - Yu, Dehong

AU - Shi, Wensheng

AU - Liu, Yun

PY - 2017

Y1 - 2017

N2 - Highly efficient visible-light catalysts are achieved through forming defect-pairs in TiO2 nanocrystals. This study therefore proposes that fine-tuning the chemical scheme consisting of charge-compensated defect-pairs in balanced concentrations is a key missing step for realizing outstanding photocatalytic performance. This research benefits photocatalytic applications and also provides new insight into the significance of defect chemistry for functionalizing materials.

AB - Highly efficient visible-light catalysts are achieved through forming defect-pairs in TiO2 nanocrystals. This study therefore proposes that fine-tuning the chemical scheme consisting of charge-compensated defect-pairs in balanced concentrations is a key missing step for realizing outstanding photocatalytic performance. This research benefits photocatalytic applications and also provides new insight into the significance of defect chemistry for functionalizing materials.

KW - photocatalysis

KW - solar energy

KW - titanium dioxide

KW - visible-light catalysts

UR - http://handle.westernsydney.edu.au:8081/1959.7/uws:39290

U2 - 10.1002/adma.201605123

DO - 10.1002/adma.201605123

M3 - Article

C2 - 28112832

SN - 0935-9648

VL - 29

JO - Advanced Materials

JF - Advanced Materials

IS - 11

M1 - 1605123

ER -

The formation of defect-pairs for highly efficient visible-light catalysts

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Keywords

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